分类： 光学 >> 量子光学 提交时间： 2023-02-19
Yali Zeng
Qingdong Ou
Lu Liu
Chunqi Zheng
Ziyu Wang
Youning Gong
Xiang Liang
Yupeng Zhang
Guangwei Hu
Zhilin Yang
Cheng-Wei Qiu
Qiaoliang Bao
Huanyang Chen
Zhigao Dai
摘要： Polaritons in polar biaxial crystals with extreme anisotropy offer a promising route to manipulate nanoscale light-matter interactions. The dynamical modulation of their dispersion is great significance for future integrated nano-optics but remains challenging. Here, we report a momentum-directed strategy, a coupling between the modes with extra momentum supported by the interface and in-plane hyperbolic polaritons, to tailor topological transitions of anisotropic polaritons in biaxial crystals. We experimentally demonstrate such tailored polaritons at the interface of heterostructures between graphene and {\alpha}-phase molybdenum trioxide ({\alpha}-MoO3). The interlayer coupling can be electrically modulated by changing the Fermi level in graphene, enabling a dynamic topological transition. More interestingly, we found that the topological transition occurs at a constant Fermi level when tuning the thickness of {\alpha}-MoO3. The momentum-directed strategy implemented by interface engineering offers new insights for optical topological transitions, which may shed new light for programmable polaritonics, energy transfer and neuromorphic photonics.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： Negative reflection and negative refraction are exotic phenomena that can be achieved by platforms such as double-negative metamaterial, hyperbolic metamaterial, and phase-discontinuity metasurface. Recently, natural biaxial van der Waals (vdW) materials, which support extremely anisotropic, low-loss, and highly confined polaritons from infrared to visible regime, are emerging as promising candidates for planar reflective and refractive optics. Here, we introduce three degrees of freedom, namely interface, crystal direction, and electric tunability to manipulate the reflection and refraction of the polaritons. With broken in-plane symmetry contributed by the interface and crystal direction, distinguished reflection and refraction such as negative and backward reflection, positive and negative refraction could exist simultaneously and exhibit high tunability. The numerical simulations show good consistency with the theoretical analysis. Our findings provide a robust recipe for the realization of negative reflection and refraction in biaxial vdW materials, paving the way for the polaritonics and interface nano-optics.
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