分类: 核科学技术 >> 核材料与工艺技术 提交时间: 2024-03-13
摘要: Cs and I can migrate through the fuel-cladding interface and accelerate the cladding corrosion process induced by the Fuel Cladding Chemical Interaction. Cr coating is an important candidate in mitigating this chemical interaction. First-principles calculations were employed to investigate the diffusion behaviors of Cs and I in Cr bulk and Cr grain boundary, aiming to reveal the microscopic mechanisms for mitigating the interaction at fuel-cladding interface. The interactions between these two fission products and Cr coating were systematically studied, and the temperature-dependent diffusion coeffcients of Cs and I in Cr were obtained using Bocquet’s oversized solute atoms model and Le Claire’s nine-frequency model, respectively. The results show that the migration barriers of Cs and I are significantly lower compared to that of Cr, and the diffusion coeffcients of Cs and I are both more than 3 orders of magnitude larger than Cr self-diffusion coeffcient within the temperature range of Generation IV fast reactors (below 1000 K), which shows the strong penetration ability of Cs and I. Meanwhile, Cs and I are more likely to diffuse along the grain boundary because of the generally low migration barriers, indicating that grain boundary serves as a fast diffusion channel for Cs and I.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: We demonstrate a robust low-loss optical interface by tiling passive (i.e., without doping of active ions) thin film lithium niobate (TFLN) and active (i.e., doped with rare earth ions) TFLN substrates for monolithic integration of passive/active lithium niobate photonics. The tiled substrates composed of both active and passive areas allow to pattern the mask of the integrated active passive photonic device at once using a single continuous photolithography process. The interface loss of tiled substrate is measured as low as 0.26 dB. Thanks to the stability provided by this approach, a four-channel waveguide amplifier is realized in a straightforward manner, which shows a net gain of ~5 dB at 1550-nm wavelength and that of ~8 dB at 1530-nm wavelength for each channel. The robust low-loss optical interface for passive/active photonic integration will facilitate large-scale high performance photonic devices which require on-chip light sources and amplifiers.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: Photon loss in optical fibers prevents long-distance distribution of quantum information on the ground. Quantum repeater is proposed to overcome this problem, but the communication distance is still limited so far because of the system complexity of the quantum repeater scheme. Alternative solutions include transportable quantum memory and quantum-memory-equipped satellites, where long-lived optical quantum memories are the key components to realize global quantum communication. However, the longest storage time of the optical memories demonstrated so far is approximately 1 minute. Here, by employing a zero-first-order-Zeeman magnetic field and dynamical decoupling to protect the spin coherence in a solid, we demonstrate coherent storage of light in an atomic frequency comb memory over 1 hour, leading to a promising future for large-scale quantum communication based on long-lived solid-state quantum memories.