分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: Plasmon-mediated superradiance for molecules around metallic nanospheres was proposed ten years ago. However, its demonstration has not been achieved yet due to the experimental difficulty of positioning molecules, and the theoretical limitation to the enhanced collective rate of low excited molecules. In this Letter, we propose that the ultrafast plasmon-mediated superradiant pulses can be observed with strongly excited methylene blue molecules standing vertically inside gold nanoparticle-on-mirror nanocavities. Our simulations indicate that in this system the molecules could interact with each other via plasmon- and free-space mediated coherent and dissipative coupling. More importantly, the coherent coupling mediated by short-ranged propagating surface plasmons cancel largely the direct dipole-dipole coupling mediated by the free-space field, and the dominated dissipative coupling mediated by relatively long-ranged gap plasmons enables the ultrafast superradiant pulses within picosecond scale. Our study opens up the possibility of studying the rich superradiant effects from the quantum emitters in a sub-wavelength volumn by engineering the plasmonic environments.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: We propose how to achieve synthetic $\mathcal{PT}$ symmetry in optomechanics without using any active medium. We find that harnessing the Stokes process in such a system can lead to the emergence of exceptional point (EP), i.e., the coalescing of both the eigenvalues and the eigenvectors of the system. By encircling the EP, both non-reciprocal optical amplification and chiral mode switching can be achieved. As a result, our synthetic $\mathcal{PT}$-symmetric optomechanics works as a topological optomechanical amplifier. This provides a surprisingly simplified route to realize $\mathcal{PT}$-symmetric optomechanics, indicating that a wide range of EP devices can be created and utilized for various applications such as topological optical engineering and nanomechanical processing or sensing.