分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: The intense terahertz (THz) pulses facilitate the observation of various nonlinear optical effects and manipulation of material properties. In this work, we report a convenient approach that can produce strong broadband terahertz pulses with center frequency tunable between 2-4 THz. The coherent THz light source with pulse energy of 1.2 microjoule can be generated from a low-cost crystalline quartz pumped by an ultrashort tilted wave-front pulse. Thanks to the wide transparent spectral window and high damage threshold, our theoretical analysis and experiment show that the optical rectification in quartz is as efficient as that in LiNbO3, but covers much broader spectral range. This work not only provides the light source that is urgently needed for nonlinear THz spectroscopy beyond 1 THz, but offers an alternative route in the selection of nonlinear optical crystals for optical frequency conversion.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: A high-sensitive DC Magneto-Optical Kerr Effect (MOKE) apparatus is described in this letter. Via detailed analysis on several dominating noise sources, we have proposed solutions that significantly lower the MOKE noise, and a sensitivity of $1.5\times10^{-7} \text{rad}/\sqrt{\text{Hz}}$ is achieved with long-term stability. The sensitivity of the apparatus is tested by measuring a wedge-shaped Ni thin film on $\text{SiO}_2$ with Ni thickness varying from 0 to 3 nm. A noise floor of $1.5\times10^{-8}$ rad is demonstrated. The possibility of further improving sensitivity to $10^{-9}$ rad via applying ac modulation is also discussed.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: The low-frequency collective excitations, which often occur in the terahertz or multi-terahertz spectral region, play an essential role in many novel emergent phenomena. Despite numerous studies in the bulk, detection of such excitations at interfaces remains challenging owing to the lack of feasible experimental techniques. Here, we show that interfacial low-frequency modes can be characterized using surface-specific nonlinear terahertz spectroscopy. This technique uses intra-pulse difference frequency mixing (DFM) process that can extend the second-order optical spectroscopy to the terahertz range. As a demonstration, the surface phonon of SrTiO3(001) at 2.8 THz was successfully measured. This surface polarization originates from the excess of oxygen vacancies or charge transfer at the interface. We have also developed an analytical procedure for remote measurement of the interfacial potential of complex oxides in a practical environment. Our method offers new opportunities for in situ studies of the low-frequency excitations at interfaces in broad disciplines.