Development of a Laser-based angle-resolved-photoemission spectrometer with sub-micrometer spatial resolution and high-efficiency spin detection

分类： 光学 >> 量子光学 提交时间： 2023-02-19

R. Z. Xu X. Gu W. X. Zhao J. S. Zhou Q. Q. Zhang X. Du Y. D. Li Y. H. Mao D. Zhao K. Huang C. F. Zhang F. Wang Z. K. Liu Y. L. Chen L. X. Yang

摘要： Angle-resolved photoemission spectroscopy with sub-micrometer spatial resolution ({\mu}-ARPES), has become a powerful tool for studying quantum materials. To achieve sub-micrometer or even nanometer-scale spatial resolution, it is important to focus the incident light beam (usually from the synchrotron radiation) using X-ray optics such as the zone plate or ellipsoidal capillary mirrors. Recently, we developed a laser-based {\mu}-ARPES with spin-resolution (LMS-ARPES). The 177 nm laser beam is achieved by frequency doubling a 355 nm beam using a KBBF crystal and subsequently focused using an optical lens with a focal length of about 16 mm. By characterizing the focused spot size using different methods and performing spatial-scanning photoemission measurement, we confirm the sub-micron spatial resolution of the system. Compared with the {\mu}-ARPES facilities based on synchrotron radiation, our LMS-ARPES system is not only more economical and convenient but also with higher photon flux (> 5E13 photons/s), thus enabling the high-resolution and high-statistics measurements. Moreover, the system is equipped with a two-dimensional spin detector based on exchange scattering at a surface-passivated iron film grown on a W(100) substrate. We investigate the spin structure of the prototype topological insulator Bi2Se3 and reveal a high spin-polarization rate, confirming its spin-momentum locking property. This lab-based LMS-ARPES will be a powerful research tool for studying the local fine electronic structures of different condensed matter systems, including topological quantum materials, mesoscopic materials and structures, and phase-separated materials.

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